Research Highlights

For the first time, researchers can turn on an electric field to manipulate molecular interactions, get them to cool down further, and start to explore collective physics where all molecules are coupled to each other.

Building on their newfound ability to induce molecules in ultracold gases to interact with each other over long distances, JILA researchers have used an electric “knob” to influence molecular collisions and dramatically raise or lower chemical reaction rates.

JILA researchers have used a state-of-the-art atomic clock to narrow the search for elusive dark matter, an example of how continual improvements in clocks have value beyond timekeeping.

A strangely shaped cloud of fermions revealed a record-fast way of cooling atoms for quantum devices.

Bringing molecules down to ultracold temperatures takes a mythic approach, but the Ye Group finds that their new scheme can hold up under tough conditions.

Using optical tweezers, the Kaufman and Ye groups at JILA have achieved record coherence times, an important advance for optical clocks and quantum computing.

New research from the Cornell Group suggests that the van der Waals universality may have limitations.

It's hard to read a clock with hands that wobble. The Ye Group has found a way to steady their optical atomic clock using a new cavity.

When the Ye group measured the total quantum state of buckyballs, we learned that this large molecule can play by full quantum rules. Specifically, this measurement resolved the rotational states of the buckyball, making it the largest and most complex molecule to be understood at this level.

Understanding chemistry requires understanding both molecules and quantum physics. The former defines the start and end of chemical reactions, the latter dictates the dynamics in between. JILA researchers now have a better understanding of both.

With the advent of the laser, the fuzzy bands glowing from atoms transformed into narrow lines of distinct color. These spectral lines became guiding beacons visible from the quantum frontier. More than a half century later, we stand at the next frontier. The elegant physics that will decode today’s mysteries (such as dark matter, dark energy, and the stability of our fundamental constants, to name a few) is still shrouded in shadows. But a new tool promises illumination. 

We all know what a tenth of a second feels like. It’s a jiffy, a snap of the fingers, or a camera shutter click. But what does 14 billion years–the age of the universe–feel like? JILA’s atomic clock has the precision to measure the age of the universe to within a tenth of a second. That sort of precision is difficult to intuit. Yet, JILA’s atomic clock, which is the most precise clock in the world, continues to improve its precision. The latest jump in precision, of nearly 50 percent, came about from a new perspective.

The reaction, at first glance, seems simple. Combustion engines, such as those in your car, form carbon monoxide (CO). Sunlight converts atmospheric water into a highly reactive hydroxyl radical (OH). And when CO and OH meet, one byproduct is carbon dioxide (CO₂) ­– a main contributor to air pollution and climate change.

Why are we here? This is an age-old philosophical question. However, physicists like Will Cairncross, Dan Gresh and their advisors Eric Cornell and Jun Ye actually want to figure out out why people like us exist at all. If there had been the same amount of matter and antimatter created in the Big Bang, the future of stars, galaxies, our Solar System, and life would have disappeared in a flash of light as matter and antimatter recombined.

Imagine A Future . . . The International Moon Station team is busy on the Moon’s surface using sensitive detectors of gravity and magnetic and electric fields looking for underground water-rich materials, iron-containing ores, and other raw materials required for building a year-round Moon station. The station’s mission: launching colonists and supplies to Mars for colonization. Meanwhile, back on Earth, Americans are under simultaneous assault by three Category 5 hurricanes, one in the Gulf of Mexico and two others threatening the Caribbean islands. Hundreds of people are stranded in the rising waters, but thanks precision cell-phone location services and robust cell-tower connections in high wind, their rescuers are able to accurately pinpoint their locations and send help immediately.

Researchers at JILA and around the world are starting a grand adventure of precisely controlling the internal and external quantum states of ultracold molecules after years of intense experimental and theoretical study. Such control of small molecules, which are the most complex quantum systems that can currently be completely understood from the principles of quantum mechanics, will allow researchers to probe the quantum interactions of individual molecules with other molecules, investigate what happens to molecules during collisions, and study how molecules behave in chemical reactions. 

In the Ye group’s new quantum simulation experiment, cold strontium atoms, which are analogs of electrons, are allowed to tunnel between the pancakes that confine the atoms with laser light. Because the atoms moving in an array of pancakes are analogs of electrons moving in solids, such studies are expected to shed light on the complex physics of metals and other solids. Credit:  The Ye group and Steve Burrows, JILA

Deborah Jin, Jun Ye, and their students wrote a review during the summer of 2016 for Nature Physics highlighting the accomplishments and future directions of the relatively new field of ultracold-molecule research. The field was pioneered by the group’s creation of the world’s first gas of ultracold potassium-rubidium (KRb) molecules in 2008.

Using frequency comb spectroscopy, the Ye group has directly observed transient intermediate steps in a chemical reaction that plays a key role in combustion, atmospheric chemistry, and chemistry in the interstellar medium. The group was able to make this first-ever measurement because frequency combs generate a wide range of laser wavelengths in ultrafast pulses. These pulses made it possible for the researchers to “see” every step in the chemical reaction of OH + CO → HOCO → CO2 + H.

The Ye group just solved a major problem for using molecular fingerprinting techniques to identify large, complex molecules: The researchers used an infrared (IR) frequency comb laser to identify four different large or complicated molecules. The IR laser-light absorption technique worked well for the first time with these larger molecules because the group combined it with buffer gas cooling, which precooled their samples to just a few degrees above absolute zero.