TY - JOUR AU - Michael Tanksalvala AU - Christina Porter AU - Yuka Esashi AU - Bin Wang AU - Nicholas Jenkins AU - Zhe Zhang AU - Galen Miley AU - Joshua Knobloch AU - Brendan McBennett AU - Naoto Horiguchi AU - Sadegh Yazdi AU - Jihan Zhou AU - Matthew Jacobs AU - Charles Bevis AU - Robert Karl AU - Peter Johnsen AU - David Ren AU - Laura Waller AU - Daniel Adams AU - Seth Cousin AU - Chen-Ting Liao AU - Jianwei Miao AU - Michael Gerrity AU - Henry Kapteyn AU - Margaret Murnane AB - Next-generation nano- and quantum devices have increasingly complex 3D structure. As the dimensions of these devices shrink to the nanoscale, their performance is often governed by interface quality or precise chemical or dopant composition. Here, we present the first phase-sensitive extreme ultraviolet imaging reflectometer. It combines the excellent phase stability of coherent high-harmonic sources, the unique chemical sensitivity of extreme ultraviolet reflectometry, and state-of-the-art ptychography imaging algorithms. This tabletop microscope can nondestructively probe surface topography, layer thicknesses, and interface quality, as well as dopant concentrations and profiles. High-fidelity imaging was achieved by implementing variable-angle ptychographic imaging, by using total variation regularization to mitigate noise and artifacts in the reconstructed image, and by using a high-brightness, high-harmonic source with excellent intensity and wavefront stability. We validate our measurements through multiscale, multimodal imaging to show that this technique has unique advantages compared with other techniques based on electron and scanning probe microscopies. BT - Science Advances DA - 2021-01 DO - 10.1126/sciadv.abd9667 IS - 5 M1 - 5 N2 - Next-generation nano- and quantum devices have increasingly complex 3D structure. As the dimensions of these devices shrink to the nanoscale, their performance is often governed by interface quality or precise chemical or dopant composition. Here, we present the first phase-sensitive extreme ultraviolet imaging reflectometer. It combines the excellent phase stability of coherent high-harmonic sources, the unique chemical sensitivity of extreme ultraviolet reflectometry, and state-of-the-art ptychography imaging algorithms. This tabletop microscope can nondestructively probe surface topography, layer thicknesses, and interface quality, as well as dopant concentrations and profiles. High-fidelity imaging was achieved by implementing variable-angle ptychographic imaging, by using total variation regularization to mitigate noise and artifacts in the reconstructed image, and by using a high-brightness, high-harmonic source with excellent intensity and wavefront stability. We validate our measurements through multiscale, multimodal imaging to show that this technique has unique advantages compared with other techniques based on electron and scanning probe microscopies. PB - American Association for the Advancement of Science PY - 2021 EP - eabd9667 T2 - Science Advances TI - Nondestructive, high-resolution, chemically specific 3D nanostructure characterization using phase-sensitive EUV imaging reflectometry UR - https://advances.sciencemag.org/content/7/5/eabd9667 VL - 7 ER -