TY - JOUR AU - Yan Zhou AU - Yuval Shagam AU - William Cairncross AU - Kia Ng AU - Tanya Roussy AU - Tanner Grogan AU - Kevin Boyce AU - Antonio Vigil AU - Madeline Pettine AU - Tanya Zelevinsky AU - Jun Ye AU - Eric Cornell AB - Cold molecules provide an excellent platform for quantum information, cold chemistry, and precision measurement. Certain molecules have enhanced sensitivity to beyond standard model physics, such as the electron’s electric dipole moment (eEDM). Molecular ions are easily trappable and are therefore particularly attractive for precision measurements where sensitivity scales with interrogation time. Here, we demonstrate a spin precession measurement with second-scale coherence at the quantum projection noise (QPN) limit with hundreds of trapped molecular ions, chosen for their sensitivity to the eEDM rather than their amenability to state control and readout. Orientation-resolved resonant photodissociation allows us to simultaneously measure two quantum states with opposite eEDM sensitivity, reaching the QPN limit and fully exploiting the high count rate and long coherence. BT - Phys. Rev. Lett. DA - 2020-02 DO - 10.1103/PhysRevLett.124.053201 N2 - Cold molecules provide an excellent platform for quantum information, cold chemistry, and precision measurement. Certain molecules have enhanced sensitivity to beyond standard model physics, such as the electron’s electric dipole moment (eEDM). Molecular ions are easily trappable and are therefore particularly attractive for precision measurements where sensitivity scales with interrogation time. Here, we demonstrate a spin precession measurement with second-scale coherence at the quantum projection noise (QPN) limit with hundreds of trapped molecular ions, chosen for their sensitivity to the eEDM rather than their amenability to state control and readout. Orientation-resolved resonant photodissociation allows us to simultaneously measure two quantum states with opposite eEDM sensitivity, reaching the QPN limit and fully exploiting the high count rate and long coherence. PB - American Physical Society PY - 2020 SE - 053201 EP - 053201 T2 - Phys. Rev. Lett. TI - Second-Scale Coherence Measured at the Quantum Projection Noise Limit with Hundreds of Molecular Ions UR - https://link.aps.org/doi/10.1103/PhysRevLett.124.053201 VL - 124 ER -