@article{12029, author = {Moritz Hofherr and S. Häuser and J. Dewhurst and Phoebe Tengdin and S. Sakshath and Hans Nembach and S. Weber and Justin Shaw and Thomas Silva and Henry Kapteyn and Mirko Cinchetti and B. Rethfeld and Margaret Murnane and Daniel Steil and B. Stadtmüller and S. Sharma and Martin Aeschlimann and Stefan Mathias}, title = {Ultrafast optically induced spin transfer in ferromagnetic alloys}, abstract = {The vision of using light to manipulate electronic and spin excitations in materials on their fundamental time and length scales requires new approaches in experiment and theory to observe and understand these excitations. The ultimate speed limit for all-optical manipulation requires control schemes for which the electronic or magnetic subsystems of the materials are coherently manipulated on the time scale of the laser excitation pulse. In our work, we provide experimental evidence of such a direct, ultrafast, and coherent spin transfer between two magnetic subsystems of an alloy of Fe and Ni. Our experimental findings are fully supported by time-dependent density functional theory simulations and, hence, suggest the possibility of coherently controlling spin dynamics on subfemtosecond time scales, i.e., the birth of the research area of attomagnetism.}, year = {2020}, journal = {Science Advances}, volume = {6}, pages = {eaay8717}, month = {2020-01}, url = {https://advances.sciencemag.org/content/6/3/eaay8717.full}, doi = {10.1126/sciadv.aay8717}, }